ITT: Excellent voice acting in video games
Also, bonus points if they did motion-capture, too.
EDIT: Videos/sound clips too, please!
Spoilers abound. You have been warned.
So I chose Majid Sadiq in Splinter Cell Blacklist, voiced by Carlo Rota. Heck, Eric Johnson's voice work as Sam isn't too bad in this scene, either... Ubisoft missed a good opportunity to create a new main protagonist for the series, but oh well.
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Vaas. Voiced, modeled, and mocaped by Michael Mando.