I loved most of ODST's soundtrack, especially the first movement of "Deference for Darkness." Can't go wrong with Marty's soundtracks. A lot of music by Jesper Kyd is good too; he's done soundtracks for a bunch of games, including Assassin's Creed [the first four games or so] and both Borderlands.
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Ah yes... The first movement to Deference for darkness... Such a beautiful piece.
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Gotta love Marty! And I do love me some of that sweet, sweet Borderlands.